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a Schematic surface composition modify by out-of-aircraft octahedral tilt in prime look at. The tilt results in a “dimer-like” structure forming by two apical I atoms through the prime of adjacent inorganic cages. b Atomic-resolution STM image in the exfoliated n = 4 RPP at Vbias = +two.three V. The device mobile is marked as being the blue rectangle Using the vector a and b. Scale bar, two nm. c Simulated charge density plot. d Schematic on the Instructions of electron tunneling in STM measurement beneath different Vbias.

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In n = 1 RPP, the BA cations interlaced with each other mainly because of the conversation with apical I atom (shaded as red) of area PbI6 octahedron, where by a larger in-airplane octahedral tilt and a small out-of-airplane tilt exist. In the case of n = four RPP, the BA molecules adopt a “head-to-head” configuration in order that their NH3 groups are positioned to get strong hydrogen bonding interactions Using the two apical I atoms of surface area PbI6 octahedron with huge out-of-airplane tilt, causing alternating very long and limited I–I distances at surface that can be viewed given that the obvious “dimer” constructions in the STM image of Fig. 3g.

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